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To better understand heat transport at the nanoscale, JILA Fellows Margaret Murnane, Henry Kapteyn, and their research groups within the STROBE NSF Center, JILA, and the University of Colorado Boulder, created the first general analytical theory of nanoscale-confined heat transport, that can be used to engineer heat transport in 3D nanosystems—such as nanowires and nanomeshes—that are of great interest for next-generation energy-efficient devices. This discovery was published in NanoLetters.

Two-dimensional materials, like graphene and 2D semiconductors, are an area of physics that has been growing tremendously in the last decade. According to JILA graduate student Ben Whetten, “That’s because they exhibit new spin and electronic physical phenomena and have much promise to build new miniaturized photonic or semiconductor nanoscale devices.” Researchers like Whetten, and his advisor, JILA Fellow, and University of Colorado Boulder professor Markus Raschke, develop methods to image these materials, giving a better understanding of their inner workings. In a new paper in NanoLetters, Raschke, and his team extended their ultrafast microscope to see nanometer-sized imperfection(s) within a 2D semiconductor sample that created some surprising nonlinear optical effects.

This year, JILA celebrates its 60th anniversary. Officially established on April 13, 1962, as a joint institution between the University of Colorado Boulder and the National Institute of Standards and Technology (NIST), JILA has become a world leader in physics research. Its rich history includes three Nobel laureates, groundbreaking work in laser development, atomic clocks, underlying dedication to precision measurement, and even competitive sports leagues. The process of creating this science goliath was not always straightforward and took the dedication and hard work of many individuals.

Functional materials—like molecular electronics, biomaterials, light-emitting diodes, or new photovoltaic materials—gain their electronic or photonic properties from complex and multifaceted interactions occurring at the elementary scales of their atomic or molecular constituents. In addition, the ability to control the functions of these materials through external stimuli , e.g., in the form of strong optical excitations, enables new properties in the materials, making them appealing for new technological applications. However, a major obstacle to overcome is the combination of the very fast time (billionths of a second) scales and the very small spatial (nanometer) scales which define the many-body interactions of the elementary excitations in the material which define its function. The extremely high time and spatial resolutions needed have been extremely difficult to achieve simultaneously. Many physicists have, therefore, struggled to visualize the interactions within these materials. In a paper recently published in Nature Communications, JILA Fellow Markus Raschke and his team report on a new ultrafast imaging technique that could solve this issue.

Physicists develop some of the most cutting-edge technologies, including new types of lasers, microscopes, and telescopes. Using lasers, physicists can learn more about quantum interactions in materials and molecules by taking snapshots of the fastest processes, and many other things. While lasers have been used for decades, their applications in technology continue to evolve. One such application is to generate and control x-ray laser light sources, which produce much shorter wavelengths than visible light. This is important because progress in developing x-ray lasers with practical applications had essentially stalled for over 50 years. Fortunately, researchers are beginning to change this by using new approaches. In a paper published in Science Advances, a JILA team, including JILA Fellows Margaret Murnane, and Henry Kapteyn, manipulated laser beam shapes to better control properties of x-ray light.

JILA Fellow Margaret Murnane has been awarded an Honorary Doctorate from the University of Limerick this year - her 6th Honorary Doctorate.

In a new paper published in Nano Letters, JILA Fellow Markus Raschke and graduate student Thomas Gray describe how they developed a way to image and visualize how surface molecules couple and interact with quantum precision. The team believes that their nanospectroscopy method could be used for molecular engineering to develop better molecular surfaces, with controlled properties for molecular electronic, photonic, or biomedical applications.

Two new papers from the Murnane and Kapteyn group are changing the way heat transport is viewed on a nanoscale, and explain the group’s surprising finding that nanoscale heat transport can be far more efficient than originally thought. One of these papers, published in the Proceedings of the National Academy of Sciences (PNAS), explains heat transport for the tiniest of hotspots, with sizes <100 nm. The other, published in American Chemical Society Nano (ACS Nano), presents a theory that is applicable to larger arrays of hotspots. Both papers postulate theories that can fully explain the surprising data collected by the team of researchers, showing that heat transport on scale lengths relevant to a wide range of nanotechnologies is more efficient than originally thought.

The Kapteyn-Murnane group has come up with a novel way to use fast bursts of extreme ultraviolet light to capture how strongly electrons interact with each other in materials. This research is important for figuring out how quickly materials can change their state from insulating to conducting, or from magnetic to nonmagnetic. In the future such fast switching may lead to faster and more efficient nanoelectronics.

Dennis Gardner and his coworkers in the Kapteyn-Murnane group accomplished two major breakthroughs in imaging tiny structures much too small to be seen with visible light microscopes: (1) for the first time in the extreme ultraviolet (EUV) or soft X-ray region, they achieved a resolution smaller than the wavelength of the light; and (2) for the first time, they obtained high resolution quantitative imaging of near periodic tiny objects (structures with repetitive features).